Cross-validated ICP-MS Methodology for Ultratrace ²³²Th/²³⁸U Determination in Material Radiopurity Assessment

26 Aug 2025, 14:20
20m
North Hall #3

North Hall #3

Oral Underground Laboratories Underground Laboratories

Speaker

Yan Zhu (Shanghai Jiao Tong University)

Description

This study established an optimized protocol employing quadrupole inductively coupled plasma mass spectrometry (ICP-QMS) with internal standard calibration to achieve direct ultratrace ²³⁸U and ²³²Th radionuclides quantification. Cross-validation with high-purity germanium gamma spectroscopy (HPGe) confirmed the method’s reliability. Systematic ICP-QMS screening of industrial materials established the current baseline radioactivity in stainless steel and titanium metals. Through UTEVA resin enrichment, ²³²Th and ²³⁸U in copper were quantified at μBq/kg-level radioactivity. Impurity profiling across smelting stages demonstrated vacuum electron beam smelting's exceptional purification efficacy.

Author

Yan Zhu (Shanghai Jiao Tong University)

Co-author

涛 张 (上海交通大学)

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